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زمین شیمی فلزات سنگین در پساب‌های ورودی و آب رودخانه کارون محدوده استان خوزستان

Name: زمین شیمی فلزات سنگین در پسابهای ورودی و آب رودخانه کارون محدوده استان خوزستان
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چکیده

زمین شیمی فلزات سنگین در پساب‌های ورودی و آب رودخانه کارون محدوده استان خوزستان

کارون طولانیترین و تنها رودخانه قابل کشتیرانی در ایران است. بسیاری از صنایع مانند صنایع فلزی، پتروشیمی و صنایع نفتی در اطراف این رودخانه قرار دارند. این رودخانه نیاز آب صنایع حاشیه خود و همچنین آب آشامیدنی شهرهایی مانند اهواز، آبادان و خرمشهر را تأمین میکند. در این مطالعه 38 نمونه آب و 28 نمونه پساب ورودی به رودخانه کارون جهت بررسی غلظت فلزات سنگینAl, As, Cd Co, Cr, Cu, Fe, Mn, Mo, Ni, Pb) Sb, Se, Zn, V , (Hg جمعآوری و تجزیه شدند. نتایج نشان داد که نمونههای آب حوضه آبریز کارون دو تیپ را نشان میدهند، به طوری که رودخانه دز تیپ بیکربنات تا سولفات و رودخانه کارون تیپ کلروره دارند. نتایج تجزیه شیمیایی نشان داد که غلظت بالای برخی فلزات در نمونههای آب رودخانه به نواحی مجاور تخلیه پساب واحدهای صنعتی و کشاورزی به رودخانه محدود میشود. مقایسه غلظت فلزات سنگین در نمونههای آب رودخانه با میانگین غلظت آنها در رودخانههای جهان نشان میدهد غلظت عناصر سرب، آهن، منگنز، وانادیم، آنتیموان و روی در منطقه مورد مطالعه افزایش یافته است. در این مطالعه مهمترین عنصر آلاینده در حوضه آبریز کارون جیوه است. به طور کلی میتوان نتیجه گرفت آلودگی به سمت خلیج فارس، افزایش می یابد.

کلید واژهها : آب، پساب ورودی به رودخانه، حوضه آبریز کارون، فلزات سنگین

دسته: فنی و مهندسی, مهندسي مکانيک برچسب: پساب ورودی به رودخانه, حوضه آبریز کارون, فلزات سنگین, کلید واژهها : آب

توضیحات
نظرات (187)

فهرست مطالب

عنوان صفحه

فصل اول: کليات و مروری بر مطالعات پیشین

1-1- مقدمه. 2

1-2- رودخانهها 3

1-3- محیط زمین شیمیایی آب و ارزیابی زیستمحیطی آن.. 3

1-4- فلزات سنگین…………………………………………………………………….5

1-4-1- منابع طبیعی ورود عناصر به محیط……………………………………… 6

1-4-2- منابع انسانزاد آلودگی فلزات سنگین.. 7

1-5- توزیع فلزات سنگین در محیط آب……………………………………………….8

1-5-1- آرسنیک… 8

1-5-2- سرب…………………………………………………………………………………..9

1-5-3- آلومینیوم……………………………………………………………………………10

1-5-4-جیوه………………………………………………………………………………….10

1-5-5-کادمیم……………………………………………………………………………… 11

1-5-6- روی………………………………………………………………………………….11

1-5-7-مس ………………………………………………………………………………….12

1-5-8-نیکل ………………………………………………………………………………..13

1-5-9-کبالت ………………………………………………………………………………..13

1 -5-10- آهن.. 14

1-5-11- کروم. 14

عنوان صفحه

1-5-12- مولیبدن……………………………………………………………………………15

1-5-13- منگنز……………………………………………………………………………….15

1-5-14- سلنیم………………………………………………………………………………..16

1-6- آنیون و کاتیونهای اصلی در آب………………………………………………………… 17

1 -6-1- کلسیم.. 17

1-6-2- منیزیم.. 17

1-6-3- سدیم……………………………………………………………………………………17

1-6-4- پتاسیم 18

1-6-5 – بیکربنات.. 18

1-6-6-کلر. 18

1-6-7- سولفات 19

1-6-8- نیترات و نیتریت… 19

1-7- مطالعات پیشین ……………………………………………………………… 19

1-8- ضرورت اجرای پژوهش 21

فصل دوم: موقعیت جغرافیایی و جغرافیایی منطقه مورد مطالعه

2-1- مقدمه. 24

2-2- ویژگیهای جغرافیایی استان خوزستان.. 25

2-2-1- اقلیم.. 25

2 -2-2- رودخانه ها …………………………………………………………….. 25

2-2-2-1- رودخانه کارون………………………………………………………………..26

2-2-2-2- رودخانه دز ………………………………………………………………….. 26

2-3- ویژگیهای آب و هوایی استان………………………………………………………… 26

2-4- صنعت……………………………………………………………………………………. 26

2-4-1- صنعت نفت… 28

عنوان صفحه

2-4-2- صنایع موجود در حاشیه رودخانه کارون.. 28

2-4-2-1- صابون سازی خرمشهر. 29

2-4-2-2-نیروگاه رامین 29

2-4-2-3- کارخانه کاغذ پارس… 30

2-4-2-4 –پالایشگاه نفت آبادان.. 30

2-4-2-5- پتروشیمی آبادان.. 31

2-4-2-6-حوضچههای پرورش ماهی.. 31

2-5- کشاورزی در خوزستان…………………………………………………………………..32

2-5-1-کشت نیشکر در خوزستان.. 34

2-6- حوضه آبریز کارون …………………………………………………………… 34

2-6-1- بخش میانی حوضه آبریز کارون…………………………………………………..37

2-6-2-بخش غربی حوضه آبریز کارون……………………………………………………38

2-7- زمین شناسی منطقه……………………………………………………………………….38

2-8- چینه شناسی منطقه مورد مطالعه………………………………………………………..40

2-8-1- چینهشناسی نواحی جنوب، غرب و جنوب شرق استان…………………………40

2-8-1-1- سازند گچساران ……………………………………………………………….41

2-8-1-2- سازند میشان……………………………………………………………………42

2-8-1-3- سازند آغاجاری……………………………………………………………….. 42

2-8-1-4- بخش لهبری …………………………………………………………………. 42

2-8-1-5- سازند بختیاری…………………………………………………………………44

2-8-1-6- نهشته های کواترنر……………………………………………………………..44

2-8-2- چینهشناسی نواحی شمال، شمال شرق و شمال غرب ………………………..45

2-8-2-1- سازند سورمه……………………………………………………………………..45

2-8-2-2- کژدمی…………………………………………………………………………….46

2-8-2-3- سروک ……………………………………………………………………………47

عنوان صفحه

2-8-2-4- سورگاه…………………………………………………………………………….47

2-8-2-5- ایلام……………………………………………………………………………….48

2-8-2-6- گورپی…………………………………………………………………………….48

2-8-2-7- پابده……………………………………………………………………………….49

2-8-2-8- آسماری…………………………………………………………………………..49

فصل سوم: مواد و روشها

3-1- مقدمه. 52

3-2- روش نمونه برداری و آماده‌سازی نمونه‌های آب و پسابهای ورودی به حوضه

آبریز کارون…………………………………………………………….57

3-3- روش‌های تجزیه‌ای 60

3-3-1- اساس کار روش ICP-MS ……………………………………………………….60

3-3-2- اندازه‌گیری کاتیون و آنیون‌های اصلی و نیترات ………………………………61

3-3-2-1- تعیین مقدار سدیم نمونه‌های آب ……………………………………… 61

3-3-2-2- تعیین مقدار پتاسیم …………………………………………………… 61

3-3-2-3- تعیین مقدار کلسیم …………………………………………………….. 62

3-3-2-4- تعیین مقدار منیزیم ……………………………………………………. 62

3-3-2-5- تعیین مقدار کلر به روش مور(mohr) ………………………………. 62

3-3-2-6- تعیین کربنات و بی‌کربنات ………………………………………………62

3-3-2-7- تعیین سولفات نمونه‌های آب …………………………………………..63

3-4- پارامترهای فیزیکی و شیمیایی مورد بررسی ………………………………. 63

3-4-1-pH…………………………………………………………………………………… 63

3-4-2- هدایت الکتریکی(Electrical Conductivity) ………………………………..64

3-4-3- TDS (Total Dissolved Solid ) ……………………………………………. 64

3-5- تحلیل دادهها 65

عنوان صفحه

3-5-1- روش‌های زمین شیمیایی تحلیل داده‌ها …………………………………….65

3-5-1-1- ضریب تمایز……………………………………………………………………. 65

3-5-1-2- سختی کل برحسب کربنات کلسیم (TH) ………………………………….66

3-5-1-3- نسبت جذب سدیم (Sodium Adsorption Ratio ) …………………….66

3-5-1-4- درصد سدیم محلول (SSP ) ………………………………………………….67

3-5-2- نمودارها 68

3-5-2-1- نمودار پایپر……………………………………………………………………….68

3-5-2-2- نمودار ویلکاکس…………………………………………………………………69

3-5-3-روشهای آماری.. 69

3-5-3-1- آمارتوصیفی ((Descriptive Statistics 70

3-5-3-2- تحلیل خوشه‌ای 70

3-5-3- 3- تحلیل مولفه‌های اصلی (PCA) 70

فصل چهارم: فلزات سنگین در آب و پسابهای ورودی به حوضه آبریز کارون

4-1- بررسی آب و پساب‌های ورودی به حوضه آبریز کارون ……………………….. 73

4-1-1- پارامترهای فیزیکوشیمیایی……………………………………………………….73

4-1-1-1- کلسیم ……………………………………………………………………….82

4-1-1-2- منیزیم ………………………………………………………………………84

4-1-1-3- پتاسیم……………………………………………………………………….85

4-1-1-4- سدیم …………………………………………………………………………86

4-1-1-5- کلر ……………………………………………………………………………88

4-1-1-6- سولفات……………………………………………………………………….89

4-1-1-7- بیکربنات …………………………………………………………………….91

4-1-1-8- نیترات ………………………………………………………………………..92

عنوان صفحه

4-1-2- نمودار پایپر ………………………………………………………………………………97

4-1-3- نمودار ویلکاکس ………………………………………………………………………100

4 -1-4- سختی آب …………………………………………………………………………….102

4-1-5- درصد سدیم محلول (SSP) ………………………………………………………….104

4-2- فلزات سنگین …………………………………………………………………….105

4-2-1- آلومینیم.. 112

4-2-2- آرسنیک……………………………………………………………………113

4-2-3- کبالت …………………………………………………………………………………115

4-2-4- مس ……………………………………………………………………………………116

4-2-5- آهن ……………………………………………………………………………………118

4-2-6- منگنز ………………………………………………………………………………….120

4-2-7- مولیبدن ………………………………………………………………………………121

4-2-8- نیکل …………………………………………………………………………………123

4-2-9- سرب …………………………………………………………………………………125

4-2-10- آنتیموان ……………………………………………………………………………126

4-2-11- سلنیم ……………………………………………………………………………..127

4-2-12- روی ………………………………………………………………………………..129

4-2-13- وانادیم ……………. ………………………………………………………………130

4-2-14- جیوه ……………………………………………………………………………….132

4-3- مقایسه میانگین غلظت عناصر آب حوضه آبریز کارون با برخی دیگر از

رودخانههای جهان…………………………………………………………..133

4-4-تحلیل داده‌ها با استفاده از روش‌های زمین شیمیایی …………………………..135

4-4-1- ضریب تمایز ……………………………………………………………….135

4-4-1-1- نمونههای آب ………………………………………………………..135

4-4-1-2- نمونههای پساب ……………………………………………………..141

عنوان صفحه

4 -4-1-3- تغییرات غلظت جیوه در نمونه های آب رودخانه و پساب…………145

4-4-2- تحلیل داده ها با استفاده از روش های آماری …………………………146

4-4-2-1- تجزیه خوشه ای (Cluster Analysis) ……………………………148

4 -4-2- 2- تحلیل مولفه اصلی (Principal Component Analysis-PCA). 151

4-4-2-3- مقایسه میانگین غلظت عناصر در آب و پساب (t- test) ……………153

فصل پنجم: نتیجه گیری و پیشنهادات

5-1- نتیجه گیری.. 156

2-5- پیشنهاد برای مطالعات آینده. 159

منابع

منابع فارسی.. 160

منابع انگلیسی.. 163

چکیده و صفحه عنوان به انگلیسی

فهرست جداول

عنوان صفحه

جدول 2-1- ‌میزان تولید برخی از محصولات کشاورزی و سهم و رتبه استان . 33

جدول 3-1- مختصات جغرافیایی و نام ایستگاههای نمونه برداری از آب

رودخانه …………………………………………………………………55

جدول3-2- مختصات جغرافیایی و نام ایستگاههای نمونهبرداری از پسابهای

ورودی به رودخانه …………………………………………………….56

جدول3-3- رده بندی کیفی آب بر حسب هدایت الکتریکی.. 64

جدول3-4- رده بندی کیفی آب شرب.. 64

جدول 3-5- تقسیمبندی آب سطحی جهت کشاورزی ………………………………65

جدول 3-6- تقسیم بندی آب بر اساس سختی ……………………………………..66

جدول3-7- رده بندی آب بر حسب SAR ……………………………………………………67

جدول 3-8- رده بندی آب بر حسب درصد سدیم …………………………………….68

جدول 4-1- غلظت یونها و پارامترهای اصلی نمونه‌های آب برداشت شده از حوضه

آبریز کارون ………………………………………………………….74

جدول 4-2- غلظت یونها و پارامترهای اصلی نمونه‌های پساب ورودی به حوضه

آبریز کارون……………………………………………………………76

جدول 4-3- خلاصه آماری پارامترهای فیزیکوشیمیایی نمونه های آب رودخانه…. 78

جدول 4-4- خلاصه آماری پارامترهای فیزیکوشیمیایی نمونه های پساب ورودی

به آب رودخانه…………………………………………………………..78

جدول 4-5- نتایج TDS نمونههای آب و پساب ورودی به رودخانه. 81

جدول 4-6- طبقه بندی آبهای سطحی جهت کشاورزی بر اساس EC و SAR 100

عنوان صفحه

جدول 4-7- SAR و EC نمونههای آب و زهکش کشاورزی ……………………….100

جدول 4-8- سختی نمونه‌های آب و پساب 103

جدول 4-9- درصد سدیم محلول نمونه‌های آب و پساب 104

جدول 4-10- غلظت برخی فلزات سنگین در نمونه‌های آب حوضه آبریز کارون…..107

جدول4-11- غلظت برخی فلزات سنگین در نمونه‌های پساب ورودی به رودخانه. 109

جدول 4-12- خلاصه آماری نمونه‌های آب حوضه آبریز کارون 111

جدول4-13- خلاصه آماری نمونه‌های پساب ورودی به آّب حوضه آبریز کارون 111

جدول4-14- مقایسه میانگین غلظت عناصر آب حوضه آبریز کارون با برخی

دیگر از رودخانههای جهان ……………………………………….. 134

جدول 4-15- آزمون نرمال بودن توزیع عناصر و یون های اصلی

و پارامترهای فیزیکوشیمیایی آب رودخانه …………………………. 147

جدول 4-16- تحلیل عاملی فلزات سنگین نمونه‌های آب …………………………..152

جدول 4-17- نتایج حاصل از مقایسه میانگین غلظت عناصر در آب

پساب (t- test)………………………………………………………………….154

فهرست اشکال

عنوان صفحه

شکل2-1- نقشه جغرافیایی محدوده مطالعاتی.. 25

شکل2-2- حوضه آبریز کارون.. 37

شکل2-3– نقشه زمین شناسی منطقه مورد مطالعه. 39

شکل3-1- موقعیت نقاط نمونه برداری از آب رودخانه 53

شکل3-2- موقعیت نقاط نمونه برداری از پساب ورودی به رودخانه. 54

شکل3-3- نمونهبرداری از آب رودخانه. 58

شکل 3-4- نمونهبرداری از پساب……………………………………………………..58

شکل 3-5- اندازهگیری پارامترهای آب………………………………………………………..59

شکل 3-6- آماده سازی نمونه های آب ………………………………………………59

شکل 3-7 تجزیه به روش ICP-MS ………………………………………………….61

شکل4-1- هدایت الکتریکی نمونه های آب رودخانه در ایستگاههای مختلف… 80

شکل4-2- غلظت کلسیم در ایستگاههای مختلف… 83

شکل4-3- نمودار هیستوگرام کلسیم …………………………………………………83

شکل4-4- تغییرات منیزیم در ایستگاههای مختلف 84

شکل4-5- نمودار هیستوگرام منیزیم 85

شکل4-6- تغییرات غلظت پتاسیم در ایستگاههای مختلف 86

شکل4-7-نمودار هیستوگرام پتاسیم.. 86

شکل4-8- تغییرات غلظت سدیم در ایستگاههای مختلف 87

شکل4-9- نمودار هیستوگرام سدیم 87

شکل4-10- تغییرات غلظت کلر در ایستگاه های مختلف… 89

شکل4-11- نمودار هیستوگرام کلر 89

عنوان صفحه

شکل4-12- تغییرات غلظت سولفات در ایستگاههای مختلف 90

شکل4-13- نمودار هیستوگرام سولفات 91

شکل4-14- تغییرات غلظت بیکربنات در ایستگاههای مختلف 92

شکل4-15- نمودار هیستوگرام بیکربنات 92

شکل4-16- تغییرات غلظت نیترات در ایستگاههای مختلف…………………………93

شکل4-17- نمودار هیستوگرام نیترات 94

شکل 4-18- نمودار افزودگی کاهیدگی یون های اصلی……………………………………95

شکل 4-19- نمودار پایپر نمونه های آب حوضه آبریز کارون …………………………98

شکل4-20- نمودار پایپر نمونه های پساب ورودی به حوضه آبریز کارون 99

شکل4-21- نمودار Wilcox 102

شک 4-22- نمودار تغییرات غلظت آلومینیوم در ایستگاههای مختلف 113

شکل4-23- نمودار هیستوگرام آلومینیم 113

شکل4-24- نمودار تغییرات غلظت آرسنیک در ایستگاه های مختلف 114

شکل4-25- نمودار هیستوگرام آرسنیک… 115

شکل4-26- نمودار تغییرات کبالت در ایستگاه‌های مختلف 116

شکل4-27- نمودار هیستوگرام کبالت 116

شکل4-28- تغییرات غلظت مس در ایستگاه‌های مختلف 118

شکل4-29- نمودار هیستوگرام مس…. 118

شکل4-30- نمودار تغییرات غلظت آهن در ایستگاه‌های مختلف 119

شکل4-31- نمودار هیستوگرام آهن 119

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امتیاز 4 از 5

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